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5,6 bond In the absence of the N atom, both of the odd-numbered p systems would be neutral with a SOMO at However, the presence of the N atom lowers the third orbital of the ve-atom part, and this orbital will be doubly occupied, leaving six electrons for the heptadienyl part Thus a formal charge separation is predicted the rotational TS consists of a heptadienyl cation and a 1-azapentadienyl anion This ``sudden polarization'' is responsible for the large change in dipole moment and hence the electrical pulse responsible for vision For a detailed experimental study of the mechanism of the isomerization, see Haran, G; Morlino, E A; Matthes, J; Callender, R H; Hochstrasser, R M, J Phys Chem A, 1999, 103, 2202 2207 Also see Kandori, H; Sasabe, H; Nakanishi, K; Yoshizawa, T; Mizukami, T; Shichida, Y, J Am.

Chronological Age (year) Height (cm)

250 200 Heating rate 10 C/min Weight left Heat flow Heating rate 50 C/min Weight left Heat flow 150 100 50 0 50 100 1000 Heat flow (mW)

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Chem Soc, 1996, 118, 1002 1005 6 1 A recent study (Seeman, J I; Grassian, V H; Bernstein, E R, J Am Chem Soc, 1988, 110, 8542) has demonstrated that -methylstyrene is nonplanar in the ground state but is planar in its rst excited state This may be interpreted as evidence that the p bond order of the bond connecting the vinyl group to the ring is greater in the lowest p p state than in the ground state Can you o er an explanation for this observation by considering the properties of styrene to arise from the interaction of a benzene ring with ethylene Answer The HOMOs and LUMOs of benzene and ethylene have the same SHMO energies, j j and j j, respectively These HOMOs interact, the out-of-phase combination becoming the HOMO of styrene.

class MyClass implements MyInterface { public function myMethod1( $param1, $param2 ) { // (implement the method here) } public function myMethod2( $param1, $param2 ) { // (implement the method here) } }

The process of network authentication can be as simple as a user ID10 and password. However, even with that, users can be restricted by their group association to certain locations or resources within the network. It is the responsibility of the client to properly identify itself to the authentication servers on the network.

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This tells you that an exception occurred that wasn t handled by the script itself, gives you the error message, and informs you that the exception was thrown in the main (top-level) part of the script.

Thus the HOMO of styrene is antibonding across the bond connecting the vinyl group to the ring Upon photoexcitation, one electron leaves this orbital, resulting in a net increase of the p bond order of this bond The LUMO of styrene corresponds to the in-phase combination of the LUMOs of ethylene and benzene and therefore contributes a positive contribution to the p bond order of the connecting bond when it receives the photoexcited electron..

3

Figure 6-3: To set a background color, after selecting the Inspector s color swatch, click the desired color.

The Site Extras tab includes Stationery pages and Components that you create. When you use the Inspector to turn a page into Stationery or a Component, it appears in the Stationery or Components folder in the second part of the Site Window and also in this tab of the palette. A pop-up menu in the bottom right switches between Stationery pads, Components, and items from the Site Window s Custom tab. (For more on Stationery, see 4; Components and the Custom tab are covered in 14.) On the QuickTime tab, you ll find everything you need to build a fully featured QuickTime masterpiece. (See 21 for more.) The Custom tab is your very own storage area. Anything you create on your page can be selected and dragged here. Once it s here, you can drag your creation to any page. This ll save you tons of redundant formatting, such as setting up tables or grids to your liking. (For instructions, see 14.) The WebObjects tab does not appear with the standard GoLive installation. If you ve added WebObjects capability by turning on the WebObjects Module under your preferences, it appears in the Objects palette. The WebObjects tab contains everything you need to use WebObjects on your page. WebObjects is a programming tool beyond the scope of this book, but if you re familiar with WebObjects, the Objects palette items will be familiar to you.